Record number :
Title of article :
Subsystem dynamics in mixed quantum–classical systems Original Research Article
Author/Authors :
Mohamad Toutounji، نويسنده , , Raymond Kapral، نويسنده ,
Issue Information :
هفته نامه با شماره پیاپی سال 2001
Pages :
From page :
To page :
Abstract :
Starting with the mixed quantum–classical Liouville equation, projection operator methods are used to derive an equation of motion for a quantum subsystem dissipatively interacting with a classical bath. The resulting generalized master equation is reduced to the Lindblad equation after making a Markovian approximation in the weak coupling limit. The bath subsystem dynamics is studied from a similar perspective. For situations where the classical subsystem consists of few degrees of freedom, or one is interested in the nature of the modifications of its dynamics as a result of coupling to a large, rapidly relaxing quantum bath, a classical analog of the Lindblad equation is derived and discussed.
Journal title :
Chemical Physics
Link To Document :